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EPR study of germanium-vacancy defects in diamonds

MetadataDetails
Publication Date2016-09-01
JournalJournal of Structural Chemistry
AuthorsVladimir A. Nadolinny, Andrey Komarovskikh, Yuri N. Palyanov, Igor N. Kupriyanov, Yuri M. Borzdov
InstitutionsNikolaev Institute of Inorganic Chemistry, V.S. Sobolev Institute of Geology and Mineralogy
Citations9

Diamonds synthesized in the Mg0.9-Ge0.1-C system at high pressure-high temperature (HPHT) conditions are investigated by the EPR and luminescence methods. A new GeV paramagnetic center with the spin S = 1 and D 3d symmetry is detected in the EPR spectra of the Ge-doped samples, along with the impurity nitrogen (Š 1) and silicon-vacancy defect KUL1 (SiV0) centers. The investigation demonstrates that this new center has a double semi-vacancy structure with the germanium atom in the center. The studied GeV center is in a neutral charge state and is assigned to the 602 nm system in the photoluminescence spectra.