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Interfacial energy barrier height of Al2O3/H-terminated (111) diamond heterointerface investigated by X-ray photoelectron spectroscopy

MetadataDetails
Publication Date2017-10-02
JournalApplied Physics Letters
AuthorsAurélien Maréchal, Y. Kato, Meiyong Liao, Satoshi Koizumi
InstitutionsNational Institute for Materials Science, National Institute of Advanced Industrial Science and Technology
Citations8

The interfacial band configuration of the high-Îș dielectric Al2O3 deposited at 120 ∘C by atomic layer deposition (ALD) on boron- and phosphorus-doped hydrogen-terminated (111) diamond was investigated. Performing X-ray photoelectron spectroscopy measurements of core level binding energies and valence band maxima values, the valence band offsets of both heterojunctions are found to be ΔEV = 1.8 eV and ΔEV = 2.7 eV for Al2O3/H(111)p and Al2O3/H(111)n, respectively. The ALD Al2O3 bandgap energy was measured from the O 1s photoelectron energy loss spectra to be EGAl2O3=7.1 eV. The interfacial band diagram configuration is found to be of type II for both Al2O3/H(111)p and Al2O3/H(111)n heterostructures having conduction band offsets of ΔEC = 0.2 eV and ΔEC = 1.1 eV, respectively. The use of doped (111) hydrogen-terminated diamond for developing future diamond metal-oxide-semiconductor field-effect transistors is discussed.