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High-mobility p-channel wide-bandgap transistors based on hydrogen-terminated diamond/hexagonal boron nitride heterostructures

MetadataDetails
Publication Date2021-12-23
JournalNature Electronics
AuthorsYosuke Sasama, Taisuke Kageura, Masataka Imura, Kenji Watanabe, Takashi Taniguchi
InstitutionsNational Institute for Materials Science, University of Tsukuba
Citations154
AnalysisFull AI Review Included

This research reports the fabrication of high-performance, normally-off p-channel wide-bandgap field-effect transistors (FETs) utilizing hydrogen-terminated diamond (H-diamond) and hexagonal boron nitride (h-BN) heterostructures.

  • Mobility Breakthrough: Achieved the highest room-temperature Hall hole mobility (680 cm2V-1s-1) reported for any p-channel wide-bandgap semiconductor FET, surpassing GaN and SiC counterparts.
  • Normally-Off Operation: Successfully demonstrated normally-off behavior (Vth = -0.99 V) with a high on/off ratio exceeding 108, crucial for fail-safe power electronics.
  • Record On-State Performance: Achieved the lowest sheet resistance (1.4 kΩ) and highest gate-length-normalized on-current (1600 ”m mA mm-1) for p-channel wide-bandgap FETs.
  • Novel Mechanism: Conductivity is generated by an inversion layer of holes induced by gate bias, eliminating the need for traditional surface transfer doping (STD) which relies on ionized surface acceptors.
  • Reduced Scattering: The air-free fabrication process significantly reduces atmospheric surface acceptors, minimizing carrier scattering and enabling the high mobility observed.
  • Cryogenic Stability: Gate controllability and high mobility are retained down to cryogenic temperatures (4.5 K), suggesting suitability for extreme environments.
ParameterValueUnitContext
Room-Temperature Hall Mobility (”Hall)680cm2V-1s-1Highest reported for p-channel wide-bandgap FETs (Device C1)
Low-Temperature Mobility>1000cm2V-1s-1Measured at 150 K (VGS = -8 V)
Minimum Sheet Resistance (ρmin)1.4kΩAt VGS = -10 V (Device C1)
Maximum Normalized On-Current (LGIDmax/WG)1600”m mA mm-1Highest reported for p-channel wide-bandgap FETs
On/Off Ratio>108-Measured at VDS = -10 V
Threshold Voltage (Vth)-0.99VConfirms normally-off (enhancement) mode operation
Maximum Hall Carrier Density (pHall)6.6 x 1012cm-2At VGS = -10 V
Minimum Subthreshold Swing (SS)130mV dec-1At VGS = -0.55 V
Interface Trap Density (Dit)6.8 x 1011cm-2eV-1Calculated from SS
Gate Leak Current Density3 x 10-7A cm-2Normalized by gate area (VGS = 0 to -10 V)
Gate-Source Breakdown Field>4.2MV/cmBased on 10 V applied across 24 nm h-BN
h-BN Gate Insulator Thickness (thBN)24nmFor devices C1 and C2
Diamond Orientation(111)-IIa-type single-crystalline diamond
Intrinsic Bulk Diamond Mobility (Phonon-limited)>2000cm2V-1s-1Room temperature (Theoretical reference)

The fabrication relies on an air-free transfer and lamination process to minimize atmospheric surface acceptors, which typically cause hole scattering and normally-on behavior in H-diamond FETs.

  1. Substrate Preparation:

    • Used IIa-type (111) single-crystalline diamond.
    • Surfaces were polished and cleaned using hydrofluoric acid and a mixture of sulfuric and nitric acid (200 °C).
    • Ti/Pt Hall-bar electrodes were deposited via electron-beam lithography.
  2. Hydrogenation and Ohmic Contact Formation:

    • Diamond was annealed in H2 gas (650 °C) and exposed to hydrogen plasma (600 °C, 10-12 min) in a CVD chamber.
    • A second hydrogenation step (600-670 °C, 10 min) was performed in a separate CVD chamber.
    • These steps formed TiC ohmic contacts and hydrogenated the diamond surface.
  3. Air-Free Transfer and Lamination (Critical Step):

    • The H-diamond was transferred directly from the CVD chamber to an Ar-filled glove box using a custom-made vacuum suitcase (pressure < 10-7 Torr for Device C1).
    • Single-crystalline h-BN (24 nm thick) was cleaved in the glove box and laminated onto the H-diamond using a dry transfer technique (completed within 3 hours of diamond transfer).
    • The sample was annealed at 300 °C in Ar for 3 hours after h-BN lamination.
  4. Gate Electrode Deposition:

    • A thin graphite crystal (Kish graphite) was transferred onto the h-BN in the glove box, followed by annealing at 300 °C for 1 hour.
  5. Device Patterning and Isolation:

    • Graphite and h-BN were etched into a Hall-bar shape using plasma generated from N2, O2, and CHF3 gases (total pressure 10 Pa).
    • The etching process converted the exposed H-diamond surface (outside the h-BN region) into an oxygen-terminated surface, providing electrical isolation.
    • Ti/Au leads and bonding pads were deposited.

The exceptional performance metrics achieved by this h-BN/diamond p-channel FET—specifically the high mobility, normally-off operation, and low sheet resistance—make diamond a highly competitive material for next-generation wide-bandgap electronics.

  • Power Electronics:

    • Low-Loss Switching: The normally-off behavior and extremely low sheet resistance (1.4 kΩ) are ideal for high-efficiency power conversion systems, reducing conduction loss and cooling requirements.
    • High-Temperature Operation: Diamond’s wide bandgap (5.47 eV) and high thermal conductivity (>2200 W m-1K-1) enable operation in harsh, high-temperature environments where SiC and GaN struggle.
  • High-Frequency and RF Applications:

    • The high hole mobility supports high-frequency operation, suitable for RF power amplifiers and high-speed switching devices.
  • Complementary Circuits (CMOS):

    • The development of a high-performance p-channel diamond FET paves the way for energy-efficient complementary circuits (CMOS) integrating p-channel diamond FETs with high-performance n-channel GaN FETs. This integration is crucial for low power consumption logic and driving circuitry.
  • Extreme Environment Electronics:

    • The retention of gate controllability and high mobility at cryogenic temperatures (down to 4.5 K) makes this technology viable for applications in outer space or specialized scientific instrumentation.
  • Diamond Material Technology (6ccvd.com relevance):

    • The reliance on high-quality, single-crystalline IIa-type (111) diamond substrates highlights the necessity of advanced CVD growth techniques for producing high-purity, low-defect materials essential for channel layers.