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Synthesis of Superconducting Boron-Doped Diamond in Carbon and Boron Solutions in Molten Gold and Copper

MetadataDetails
Publication Date2023-09-01
JournalInorganic Materials
AuthorsЕ. А. Екимов, V. A. Sidorov, Р. А. Хмельницкий, S. G. Lyapin
InstitutionsP.N. Lebedev Physical Institute of the Russian Academy of Sciences, Institute for High Pressure Physics

The Au-B-C and Cu-B-C growth systems, which do not form borides, have been used for the first time for the synthesis of boron-doped superconducting diamond. In these systems, the graphite-to-diamond transformation occurs at pressures from 8 to 9 GPa and temperatures from 1620 to 1770 K, suitable for commercial-scale production. The presence of boron in melts is assumed to be responsible for the decrease in synthesis temperature in molten copper and the diamond-forming ability of gold-based melts. The synthesized diamond exhibits metallic behavior of conductivity at ordinary temperatures and undergoes a superconducting transition between 4.5 and 2.5 K.