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Processing of Single Crystal Diamond (1 0 0) Plane Using Wear with Ferrous Disk

MetadataDetails
Publication Date2024-01-04
JournalJournal of the Japan Society for Precision Engineering
AuthorsGo KADO, Takeshi NAKAMOTO
AnalysisFull AI Review Included

This research presents a novel, non-mechanical method for processing single-crystal diamond (SCD) (100) surfaces by utilizing controlled thermal chemical wear against a rotating ferrous disk.

  • Core Achievement: Successful transfer of the ferrous disk’s circumferential shape, creating precise grooves on the SCD (100) face.
  • Mechanism Validation: The processing relies on the thermal chemical reaction (graphitization and carbon diffusion into the ferrous metal), confirmed by measured temperatures exceeding 700 °C during operation.
  • Material Efficiency: Ferrous disks (SK85 steel) demonstrated significantly higher processing volume compared to non-ferrous brass disks (C2801), validating the necessity of the iron-carbon reaction.
  • Shape Fidelity: A critical burr correction apparatus was developed and implemented to continuously remove burrs forming on the ferrous disk, ensuring the resulting diamond groove maintained a near-rectangular profile.
  • Surface Quality: Raman spectroscopy confirmed the high quality of the processed diamond surface and subsurface (up to 15 ”m depth), detecting only the diamond peak (1332 cm-1) and confirming the absence of residual graphite or amorphous carbon.
  • Process Control: Processing volume was shown to be highly dependent on processing time and circumferential speed, indicating the thermal nature of the removal process.
ParameterValueUnitContext
Diamond Orientation(100)-Single crystal plane processed
Diamond Dimensions2.8 x 2.5mm x mmPlane size
Ferrous Disk MaterialSK85-High hardness steel (HV 180, 0.83% C)
Non-Ferrous Disk MaterialC2801-Brass (HV 119, 0% C)
Disk Thickness0.3mmDetermines groove width
Circumferential Speed (Tested Range)250 - 500m/minProcessing parameter
Feed Rate (Tested Range)0.5 - 1.5”m/sProcessing parameter
Max Measured Temperature~700°CDiamond/Holder interface (SK85 disk)
Graphitization Temperature>600°CTemperature at which graphitization begins
Diamond Raman Peak1332cm-1Confirmed on processed surface
Raman Laser Wavelength532nmUsed for surface analysis
Raman Depth AnalysisUp to 15”mDepth analyzed for carbon residue
Required Groove Shape CorrectionBurr removal-Necessary for achieving rectangular profile
  1. Processing Setup: A single-crystal diamond (100) face was mounted in a holder, insulated from the holder using paper to minimize heat conduction and maximize the temperature rise at the contact interface.
  2. Wear Mechanism Application: A thin (0.3 mm) rotating ferrous disk (SK85) was pressed against the diamond surface and fed laterally at controlled rates (0.5 to 1.5 ”m/s) to induce localized high-temperature, high-pressure wear.
  3. Shape Transfer Verification: The disk was intentionally offset (under shift or upper shift) relative to the diamond center to confirm that the resulting groove profile on the diamond accurately reflected the shape and position of the disk’s circumference.
  4. Burr Management: A specialized correction apparatus, utilizing two grinding stones, was implemented to continuously remove burrs (バăƒȘ) that formed on the outer edge of the ferrous disk during processing. This step was critical for maintaining a precise, near-rectangular groove shape.
  5. Thermal Measurement: A K-type thermocouple (100 ”m diameter) was placed between the diamond and the holder to monitor the temperature rise, confirming that the contact zone reached temperatures sufficient for diamond graphitization (>700 °C).
  6. Surface Integrity Analysis: Post-processing analysis was performed using Raman spectroscopy. Measurements were taken at the groove base, both on the surface and in depth (up to 15 ”m), to verify the absence of graphitized carbon (peak shift to 1600 cm-1) or amorphous carbon (broadening of the Raman band).

This method offers a non-mechanical pathway for creating complex, high-fidelity shapes on diamond, addressing limitations in traditional grinding and polishing.

  • Precision Diamond Tooling: Fabrication of complex geometries (e.g., micro-grooves, specific radii) on single-point diamond cutting tools, improving performance and lifetime in ultra-precision machining of non-ferrous metals.
  • Micro-Optics and Photonics: Creation of structured surfaces, such as micro-lenses, Fresnel lenses, or diffraction gratings, directly onto diamond windows or substrates, leveraging diamond’s transparency and hardness.
  • Diamond Heat Spreaders: Shaping and patterning of diamond heat sinks for high-power density electronic devices (e.g., 5G/6G RF components, power converters) to optimize thermal pathways and bonding interfaces.
  • Microfluidics and Bio-MEMS: Etching precise, damage-free micro-channels and reservoirs into diamond substrates for chemically inert and robust microfluidic devices.
  • Advanced Wear Parts: Manufacturing diamond components requiring specific surface textures or grooves for reduced friction or enhanced lubrication in extreme environments.
View Original Abstract

Diamond has the highest hardness of all materials, high thermal conductivity and excellent optical transparency. However, it is very difficult to process the shape of the diamond because of its high hardness. By the way, when a ferrous material is cut by a diamond, the diamond is worn in spite of the diamond is much harder than the ferrous material. This phenomenon is called as thermal chemical reaction and occurs when the diamond is contacted with the ferrous material under high temperature and high pressure. This thermal chemical reaction is thought that results from the graphitization of diamond, the rapid diffusion of carbon atoms into the ferrous metal and others. In this research work, the worn due to the thermal chemical reaction was utilized diamond processing. A single crystal diamond is worn with a thin ferrous disk. This processing method was using the reactions at the interface of the diamond and the ferrous material, so the shape of the ferrous material of the contact surface can be expected to be transferred to the diamond. As a result, the diamond was grooved by the ferrous disk. Temperature of diamond during processing was measured using a K-type thermocouple. The diamond had reached the graphitization temperature. Raman spectroscopy was used to confirm if there is graphite on the diamond. Graphite was not detected on the diamond surface after processing, and only diamond peaks were detected.