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Control of spontaneous emission rate in luminescent resonant diamond particles

MetadataDetails
Publication Date2018-01-01
JournalJournal of Physics Conference Series
AuthorsRoman S. Savelev, Anastasia Zalogina, S. I. Kudryashov, Anastasia Ivanova, A. V. Levchenko
InstitutionsP.N. Lebedev Physical Institute of the Russian Academy of Sciences, Australian National University
Citations3

We study the properties of luminescent diamond particles of different sizes (up to ~1.5 μm) containing multiple NV-centers. We theoretically predict that the average liftetime in such particles is decreased by several times as compared to optically small subwavelength nanodiamonds. In our experiments, samples were obtained by milling the plasma-enhanced chemical vapor deposited diamond film, and characterized by Raman spectroscopy and dark- field spectroscopy methods. Time-resolved luminescence measurements of the excited state of NV-centers showed that their average lifetime varies from 10 to 17 ns in different samples. By comparing this data to the values of the lifetime of the NV-centers in optically small nanodiamonds, known from literature, we confirm a severalfold decrease of the lifetime in resonant particles.