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Effect of the Gas Chemistry, Total Pressure, and Microwave Power on the Grain Size and Growth Rate of Polycrystalline Diamond Films Grown by Microwave Plasma Chemical Vapor Deposition Technique

MetadataDetails
Publication Date2019-10-01
Journal2019 7th International Engineering, Sciences and Technology Conference (IESTEC)
AuthorsPablo Tirado, Jesús Alcántar, Elida de Obaldía, Rafael García, Orlando Auciello
InstitutionsUniversidad Tecnológica de Panamá, Center for Engineering and Industrial Development
Citations3

The combined effect of total gas pressure (20-80 mbar), precursor gas chemistry (Ar/CH <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;4&lt;/sub> /H <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;2&lt;/sub> ) and microwave power on the grain size and growth rate of polycrystalline diamond films, grown by MPCVD, was investigated. The key findings are: 1) Grain size of polycrystalline diamond films depends critically on the total gas pressure such that a minimum pressure of 60 mbar is needed to grow nanocrystalline diamond films (grain size of 100s of nanometers) even when using a hydrogen rich gas chemistry (98% H <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;2&lt;/sub> , 2% CH <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;4&lt;/sub> ); 2) For a fixed gas pressure, the grain size of polycrystalline diamond films increases as the H <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;2&lt;/sub> concentration increases, and decreases as the Ar concentration decreases, resulting in a maximum grain size for Ar 0%/CH <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;4&lt;/sub> 2%, H <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;2&lt;/sub> 98% gas mixture and a minimum grain size for Ar 98%/CH <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;4&lt;/sub> 2%, H <sub xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”&gt;2&lt;/sub> 0% gas mixture; 3) The microwave power (1900-2500 W) effect on grain size and growth rate.

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