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Preparing Multipartite Entangled Spin Qubits via Pauli Spin Blockade

MetadataDetails
Publication Date2020-02-26
JournalScientific Reports
AuthorsSinan Bugu, Fatih Özaydin, T. Ferrus, Tetsuo Kodera
InstitutionsTokyo Institute of Technology, Tokyo International University
Citations22
AnalysisFull AI Review Included
  • Cavity-Free W State Preparation: The research proposes a novel, solid-state scheme for preparing large-scale multipartite entangled W states using electron spins in a Double Quantum Dot (DQD) system, eliminating the need for complex photon assistance or optical cavities.
  • Pauli Spin Blockade (PSB) Fusion: The core mechanism uses PSB to verify the successful fusion of two smaller W states (Wn and Wm) into a larger state (Wn+m-2). Fusion occurs only when the two input electrons have anti-parallel spins, resulting in the absence of PSB.
  • Detection Method: Successful fusion (absence of PSB) is detected rapidly via standard transport measurement or radio-frequency reflectometry (RF-SET), relying on well-known charge sensing techniques.
  • Enhanced Success Rate: An improved setup incorporates a Toffoli gate and a CNOT gate, along with an ancillary spin-down electron, applied before the DQD. This enhancement converts the initial “failure” cases (parallel spin inputs) into successful fusion outcomes, significantly boosting the overall efficiency.
  • Industry Compatibility: The scheme is based entirely on electron spin manipulation in semiconductor DQDs, recognized as the most reliable and industry-compatible platform for scalable quantum information processing.
  • Scalability: The fusion approach allows for the progressive creation of arbitrarily large W states by iteratively fusing smaller components.
ParameterValueUnitContext
DQD Spin Coherence TimeTens ofmsAchieved in optimized DQD systems (e.g., Silicon).
QD Spin Coherence TimeFew tens of”sTypical coherence time for single quantum dots.
Electron Injection TimeFew hundreds ofpsTime required for electrons to tunnel into the DQD.
PSB Sensing Time (RF Reflectometry)FewnsFast measurement technique for spin state determination.
PSB Sensing Time (Standard)Few hundreds ofnsTypical time for transport measurement methods.
Fusion Fidelity (Noisy Setup)(1-p)2 + p2DimensionlessWhere p is the probability of an electron spin flip during the process.
Minimum Fusible W State Size (Basic)3QubitsRequired for the initial fusion setup (W3 + W3).
Minimum Fusible W State Size (Enhanced)2QubitsAchieved using the Toffoli+CNOT enhancement (allows fusion of EPR pairs, W2).
Preferred Material PlatformSilicon (Si)N/APreferred over III-V materials due to generally negligible Spin-Orbit Coupling (SOC) and non-zero nuclear spin moments.
  1. Initial State Preparation: Two W states (WA of n electrons and WB of m electrons) are prepared in quantum memories. The goal is to fuse these into Wn+m-2.
  2. Electron Injection: A single electron is extracted from WA and sent to Dot 1, and a single electron from WB is sent to Dot 2 via side injection contacts (A and B).
  3. DQD Tuning and PSB Regime: The DQD is electrostatically tuned using side gates (Vsg1, Vsg2) to operate in the Pauli Spin Blockade (PSB) regime. This regime ensures that inter-dot tunneling (current flow) is blocked if the two electrons have parallel spins (triplet state, T(1, 1)) but allowed if they have anti-parallel spins (singlet state, S(1, 1)).
  4. Spin State Determination via Charge Sensing: The presence or absence of PSB is measured using a charge sensor (e.g., radio-frequency single-electron transistor, RF-SET) or standard transport measurement, determining the spin configuration of the two electrons in the DQD.
  5. Fusion Outcome Logic:
    • Success: Absence of PSB (anti-parallel spins, ↓↑ or ↑↓) implies successful fusion, yielding Wn+m-2.
    • Recycle: Presence of PSB (parallel spins, ↓↓) implies the states are kept intact but reduced in size (Wn-1, Wm-1).
    • Failure: Presence of PSB (parallel spins, ↑↑) implies the W states collapse to separable spin-down states.
  6. Enhanced Fusion Mechanism (Optional): To improve success probability, the two input electrons and an ancillary spin-down electron are passed through a Toffoli gate followed by a CNOT gate before entering the DQD. This logic operation ensures that the initial “failure” case (↑↑) is converted into a successful fusion outcome, increasing the final state size by one qubit (Wn+m-1).

The proposed methodology directly supports the development of scalable quantum hardware, particularly within the solid-state domain:

  • Semiconductor Quantum Processors: Provides a fundamental building block for generating complex entangled states necessary for universal quantum computation, leveraging established semiconductor fabrication techniques (e.g., Si/SiGe heterostructures).
  • Quantum Repeaters and Networks: The fusion scheme is essential for creating long-distance entanglement by linking smaller entangled segments, forming the basis for robust quantum communication infrastructure.
  • High-Fidelity Qubit Control Systems: The reliance on fast, high-fidelity gate operations (Toffoli, CNOT) and rapid charge sensing (ns timescale) drives requirements for advanced, low-noise cryogenic control electronics and pulse sequencing hardware.
  • Quantum Memory Devices: Since the W states are encoded in electron spins within DQDs, which exhibit long coherence times, this preparation method is optimized for generating entangled states intended for long-term quantum information storage.
  • Advanced Metrology and Sensing: The core technique of PSB sensing, often implemented using RF-SETs, is a highly sensitive method for detecting single-electron charge and spin states, applicable to high-precision quantum sensing applications.
View Original Abstract

Abstract Preparing large-scale multi-partite entangled states of quantum bits in each physical form such as photons, atoms or electrons for each specific application area is a fundamental issue in quantum science and technologies. Here, we propose a setup based on Pauli spin blockade (PSB) for the preparation of large-scale W states of electrons in a double quantum dot (DQD). Within the proposed scheme, two W states of n and m electrons respectively can be fused by allowing each W state to transfer a single electron to each quantum dot. The presence or absence of PSB then determines whether the two states have fused or not, leading to the creation of a W state of n + m − 2 electrons in the successful case. Contrary to previous works based on quantum dots or nitrogen-vacancy centers in diamond, our proposal does not require any photon assistance. Therefore the ‘complex’ integration and tuning of an optical cavity is not a necessary prerequisite. We also show how to improve the success rate in our setup. Because requirements are based on currently available technology and well-known sensing techniques, our scheme can directly contribute to the advances in quantum technologies and, in particular in solid state systems.