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Low-temperature direct bonding of InP and diamond substrates under atmospheric conditions

MetadataDetails
Publication Date2021-05-27
JournalScientific Reports
AuthorsTakashi Matsumae, Ryo Takigawa, Yuichi Kurashima, Hideki Takagi, Eiji Higurashi
InstitutionsKyushu University, National Institute of Advanced Industrial Science and Technology
Citations15
AnalysisFull AI Review Included

This research demonstrates a robust, low-temperature method for directly bonding Indium Phosphide (InP) substrates to diamond heat spreaders, critically addressing thermal management issues in high-performance InP devices.

  • Core Achievement: Successful direct bonding of InP (100) to diamond (111) substrates achieved through surface activation and low-temperature annealing (250 °C).
  • Thermal Management: The technique utilizes diamond (2200 W/mK) to replace the low thermal conductivity InP (68 W/mK) substrate, enabling efficient heat dissipation for high-power density devices.
  • Bonding Interface Quality: The substrates are bonded via an ultra-thin (~3 nm) amorphous intermediate layer composed of In, P, O, and C, avoiding the high thermal resistance associated with conventional thick metal bonding layers (2-4 ”m).
  • Mechanical Strength: The resulting bond exhibits a shear strength of 9.3 MPa, which meets standard die shear strength requirements (MIL STD 883E).
  • Process Simplicity: The method relies on standard industrial processes: NH3/H2O2 cleaning for diamond and oxygen plasma activation for InP, followed by annealing under atmospheric conditions.
  • Surface Requirements: Both surfaces maintained atomic smoothness (RMS roughness < 3.1 A) after activation, confirming suitability for direct bonding.
ParameterValueUnitContext
Bonding Temperature250°CLow-temperature annealing step
Annealing Duration24hTime under load
Applied Load (Annealing)~1MPaPressure applied during annealing
Bond Shear Strength9.3MPaMeasured on 3x3 mm2 diamond die
Intermediate Layer Thickness~3nmAmorphous layer at InP/Diamond interface (TEM analysis)
InP Thermal Conductivity68W/mKReference value (low thermal dissipation)
Diamond Thermal Conductivity2200W/mKReference value (highest thermal conductivity solid)
InP RMS Roughness (Before O2)2.76 ± 0.3AAtomic Force Microscopy (AFM) measurement
InP RMS Roughness (After O2)3.03 ± 0.3AActivated surface condition (required < 5 A)
InP Wafer Thickness500”mStarting substrate thickness
Diamond Substrate Size3 x 3mm2Die size used for bonding test

The direct bonding process involves surface preparation to generate hydroxyl (OH) groups, followed by contacting and low-temperature thermal annealing.

StepSubstrateProcess/Recipe ParameterResult/Purpose
1. Diamond CleaningDiamond (111)Cleaned for 10 min at 75 °C using a mixture of 10 mL NH3 (28%), 10 mL H2O2 (35%), and 50 mL DI water.Generates C-OH groups (OH-termination) on the diamond surface.
2. InP ActivationInP (100)Activated using Reactive Ion Etching (RIE) with O2 plasma.Plasma parameters: 200 W power, 30 s duration, 60 Pa O2 pressure, 20 mL/min O2 flow. Generates In-OH/P-OH groups.
3. ContactingBothInP substrate cooled to 14 °C (Peltier cooler) for ~30 s, then diamond placed on InP in a clean room (23 °C, 40% RH).Cooling promotes condensed water molecules, facilitating initial hydrogen bond networks between the surfaces.
4. Annealing (Bonding)SpecimenAnnealed at 250 °C for 24 h under a load of approximately 1 MPa.Thermal dehydration reaction forms covalent atomic bonds (InP-O-C-Diamond) across the interface.
5. Interface AnalysisSpecimenTEM and EDX analysis performed after grinding InP thickness down to 10 ”m.Confirmed 3 nm amorphous layer composed of In, P, O, and C, and absence of cracks or nanovoids.

This low-temperature direct bonding technology is crucial for manufacturing next-generation devices requiring high power density and superior thermal management.

  • High-Frequency Electronics:
    • Application: Fabrication of InP High Electron Mobility Transistors (HEMTs) and Heterojunction Bipolar Transistors (HBTs) designed for THz monolithic integrated circuits (TMICs).
    • Benefit: Enables sustained high-frequency operation (fmax > 1 THz) by effectively removing localized heat, preventing performance degradation and failure.
  • High-Power RF/Microwave Devices:
    • Application: High-power InP-based amplifiers and microwave power transistors.
    • Benefit: Provides a robust, low-thermal-resistance path to the diamond heat spreader, allowing for increased power density and improved reliability compared to devices bonded with conventional metal layers.
  • Photonic Integrated Circuits (PICs):
    • Application: Integration of InP lasers, modulators, and photodetectors for next-generation optical communications systems (e.g., 1.55 ”m systems).
    • Benefit: Mitigates temperature-induced wavelength shifts and efficiency drops in high-power optical components, crucial for miniaturization and high-power operation.
  • Heterogeneous Integration:
    • Application: Wafer-level bonding of III-V semiconductors (like InP) onto high-thermal-conductivity materials (like diamond) using scalable, low-temperature processes.
    • Benefit: Simplifies manufacturing by utilizing standard cleaning and atmospheric annealing steps, contributing to higher integration density and lower manufacturing costs for advanced semiconductor devices.