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Theoretical calculation of fiber cavity coupling silicon carbide membrance

MetadataDetails
Publication Date2022-01-01
JournalActa Physica Sinica
AuthorsJi-Yang Zhou, Qiang Li, Jin‐Shi Xu, Chuan‐Feng Li, Guang‐Can Guo
AnalysisFull AI Review Included
  • Core Value Proposition: Theoretical modeling of a Fiber Fabry-Perot Cavity (FFPC) coupled to a Silicon Carbide (SiC) membrane to significantly enhance the weak infrared fluorescence of SiC spin color centers (divacancies, VSiVC).
  • Target Emitter: The PL6 divacancy center in 4H-SiC, chosen for its favorable Zero-Phonon Line (ZPL) at 1038 nm, which minimizes loss in standard optical fibers (0.7 dB/km).
  • Cavity Mode Analysis: Identified two distinct modesā€”ā€œair-modeā€ and ā€œmembrane-mode.ā€ The ā€œmembrane-modeā€ generally provides superior Purcell enhancement (β factor) but is highly sensitive to surface quality.
  • Dominant Limiting Factor: Environmental vibration (dta) is confirmed as the primary constraint on achievable cavity finesse and enhancement, especially in open FFPC systems.
  • Design Requirements: To achieve optimal enhancement using the ā€œmembrane-mode,ā€ the SiC membrane surface roughness must be maintained at less than 0.3 nm, and active/passive vibration stabilization must limit movement to less than 0.01 nm standard deviation.
  • Practical Guidance: Provides specific calculations for the optimal mirror transmission (T0) required to maximize the total outcoupling efficiency (βvib) based on the measured level of environmental vibration.
ParameterValueUnitContext
Host Material4H-SiCN/AMaterial containing VSiVC color centers.
Target Color CenterPL6 DivacancyN/ASpin-1 (S=1) quantum emitter.
ZPL Wavelength (PL6)1038nmInfrared wavelength suitable for fiber transmission.
SiC Refractive Index (nm)2.6N/AUsed for calculating mode structure.
Debye-Waller Factor (β0)3%N/ARatio of ZPL emission to total fluorescence (used for calculation).
Required Membrane Roughness (σMA)< 0.3nmNecessary for effective ā€œmembrane-modeā€ coupling.
Optimal Vibration Standard Deviation (σvib)< 0.01nmRequired for maximizing enhancement in high-finesse cavities.
Typical Membrane Thickness (tm)~4µmThickness range used in weak coupling regime calculations.
Fiber Transmission Loss (1038 nm)0.7dB/kmLoss rate for SiC ZPL photons in standard fiber.
Fiber Transmission Loss (637 nm)8dB/kmLoss rate for Diamond NV ZPL photons (for comparison).
FFPC Finesse Target> 10000N/ALong-term goal for achieving strong coupling regime.

The study employed theoretical modeling, primarily using the transmission matrix model and coupled Gaussian beam analysis, to characterize the FFPC-SiC membrane system:

  1. Cavity Mode Determination: The transmission matrix model was used to calculate the resonant frequencies (ν) and field distributions, confirming the existence and characteristics of the mixed ā€œair-modeā€ and ā€œmembrane-mode.ā€
  2. Purcell Enhancement Calculation: The Purcell factor (FP) and the ZPL coupling efficiency (β) were derived using the calculated effective cavity length (Leff), mode volume (V), and the overlap between the emitter dipole and the cavity field.
  3. Loss Analysis and Optimization: Mirror loss (LM,eff) and scattering loss (LS,eff) from the membrane surface roughness were quantified. Optimization focused on minimizing LS,eff by ensuring the membrane roughness (σMA) was sufficiently low, particularly when operating in the sensitive ā€œmembrane-mode.ā€
  4. Vibration Modeling: Environmental vibration (dta, change in air gap length) was introduced into the model using a Gaussian distribution (standard deviation σvib) to calculate the vibration-limited coupling factor (βvib).
  5. Outcoupling Efficiency Optimization: The total outcoupling efficiency (ηo = T0/Leff) was analyzed. The optimal mirror transmission (T0) was determined by finding the maximum βvib for various vibration levels, providing a trade-off between high finesse (low T0) and robustness against vibration.
  6. Future Experimental Guidance: The results guide future fabrication efforts, recommending chemical-mechanical polishing (CMP) and inductively coupled plasma (ICP) etching to achieve membrane thickness < 1 µm and roughness < 0.3 nm.

The theoretical framework developed here directly supports the engineering and deployment of next-generation quantum technologies based on solid-state emitters:

  • Quantum Communication and Networking: The use of SiC emitters at 1038 nm enables the creation of quantum repeaters and nodes compatible with existing, low-loss optical fiber infrastructure (0.7 dB/km loss).
  • Distributed Quantum Computing: Enhanced ZPL emission facilitates high-fidelity, high-rate spin-photon entanglement, a prerequisite for linking remote quantum processors.
  • High-Performance Quantum Sensing: Miniaturized FFPC-coupled SiC systems can be integrated into compact devices for advanced magnetic or electric field sensing, particularly in cryogenic or harsh environments.
  • Integrated Quantum Photonics: The FFPC design, which integrates collection and filtering directly into the fiber, is a key step toward scalable, integrated quantum light sources, avoiding the bulk and alignment issues of traditional free-space optics.
  • Quantum Light Source Development: Provides the necessary design parameters (roughness, T0, vibration tolerance) for manufacturing high-brightness, narrow-linewidth single-photon sources based on SiC divacancies.
View Original Abstract

Single spin color centers in solid materials are one of the promising candidates for quantum information processing, and attract a great deal of interest. Nowadays, single spin color centers in silicon carbide, such as divacancies and silicon vacancies have been developed rapidly, because they not only have similar properties of the NV centers in diamond, but also possess infrared fluorescence that is more favorable for transmission in optical fiber. However, these centers possess week fluorescence with broad spectrum, which prevents some key technologies from being put into practical application, such as quantum key distribution, photon-spin entanglement, spin-spin entanglement and quantum sensing. Therefore, optical resonator is very suitable for coupling centers to filter their spectrum and enhance the fluorescence by Purcell effect. It is very advantageous to use the fiber end face as cavity mirrors, thereby the fiber can provide small cavity volume corresponding to a large enhancement in spin color centers, and collect the fluorescence in cavity simultaneously, which has no extra loss in comparison with other collection methods. In this work, the properties and performance of fiber Fabry-Perot cavity coupling silicon carbide membrane are mainly studied through theoretical calculation. Firstly, some parameters are optimized such as membrane roughness and mirror reflection by calculating the mode of the fiber cavity and enhancing the color centers coupling into the cavity, then analyzing the properties of different modes in cavity, the enhancement effect on cavity coupling color centers, and other relevant factors affecting the cavity coupling color centers. Next, the influences of dominated factor and vibration on the properties of the cavity, the enhancement and outcoupling of centers coupled into the cavity are investigated, and finally the optimal outcoupling efficiency corresponding to different vibration intensities is obtained. These results give direct guidance for the further experimental design and direction for optimization of the fiber cavity coupling color centers.