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Quantum Fisher information measurement and verification of the quantum Cramér–Rao bound in a solid-state qubit

MetadataDetails
Publication Date2022-05-12
Journalnpj Quantum Information
AuthorsMin Yu, Yu Liu, Pengcheng Yang, Musang Gong, Qingyun Cao
InstitutionsMax Planck Institute for the Physics of Complex Systems, Université Libre de Bruxelles
Citations63
AnalysisFull AI Review Included

This analysis focuses on the experimental demonstration of optimal phase estimation using a solid-state Nitrogen-Vacancy (NV) center qubit, specifically verifying the saturation of the Quantum Cramér-Rao Bound (QCRB).

  • Core Achievement: Experimentally demonstrated near-saturation of the QCRB for phase estimation in a solid-state spin system (NV center in diamond), confirming optimal sensor performance.
  • Methodological Innovation: The Quantum Fisher Information (QFI)—the fundamental limit of precision—was measured independently of the estimation process using spectroscopic responses to weak parametric modulations.
  • Scalability Advantage: This technique avoids the stringent requirements of full quantum-state tomography, offering a versatile and scalable approach for characterizing QFI in more complex, multi-qubit systems.
  • QFI Extraction: QFI was directly extracted from the effective Rabi frequency (νe) induced by the parametric modulation, circumventing the need to measure state fidelity or distance between adjacent quantum states.
  • QCRB Verification: The measurement sensitivity (δβ) was shown to be linearly proportional to the inverse square root of the measured QFI (1/sqrt(Fβ)), confirming the theoretical limit.
  • Generalization: The protocol was shown to be applicable to coupled-qubit systems (NV center coupled to a 13C nuclear spin), linking high QFI values to strong entanglement near level anticrossings.
ParameterValueUnitContext
Qubit SystemNitrogen-Vacancy (NV) CenterN/ASolid-state spin system in diamond
Qubit Sublevels Usedms = 0, ms = -1N/AGround state encoding for the two-level system
External Magnetic Field (Bz)~510GApplied along the NV axis to lift spin degeneracy
Zero-Field Splitting (D)2π * 2.87GHzIntrinsic energy gap of the NV center
Initialization Laser Wavelength532nmGreen laser pulse used for spin polarization
Estimated State Fidelity>95%Purity of the prepared quantum state (evidenced by agreement with theoretical predictions)
Parametric Modulation Amplitude (aβ)0.1N/AUsed in the resonant transition measurement (Fig 2c)
Modulation Frequency (ξ)2π * 5.025MHzUsed during the parametric modulation step
Optimal Measurement Angle (α)π/2RadiansProjective measurement basis for achieving maximal sensitivity
QCRB Proportionality Factor1.041 ± 0.036N/AExperimentally measured factor verifying δβ is proportional to 1/sqrt(Fβ)
Coupled Qubit Hyperfine Coupling (Aparallel)2π * 2.79MHzUsed in numerical simulation for the NV-13C coupled system

The experiment combines standard Ramsey interferometry for phase estimation with a novel spectroscopic technique based on parametric modulation for independent QFI measurement.

  1. NV Center Initialization:

    • The NV center spin is polarized into the ms = 0 state using a 532 nm green laser pulse.
    • An external magnetic field (Bz ~ 510 G) is applied to define the ms = 0 and ms = -1 sublevels as the effective qubit.
  2. Resource State Preparation (Yθ):

    • A microwave pulse (Yθ) rotates the spin by an angle θ, preparing the initial coherent superposition resource state |ψθ(0)>.
  3. Phase Encoding (Interrogation):

    • The system undergoes free evolution for a time T, resulting in the final state |ψθ(β)>, where the phase parameter β = ξT is encoded.
  4. QFI Measurement via Parametric Modulation:

    • The system is subjected to a time-periodic parametric modulation described by the Hamiltonian H[β(t)] = H(β + aβ cos(ωt)), where aβ is small (aβ « 1).
    • Resonance Identification: The modulation frequency (ω) is swept to find the resonant condition (ω ≈ A), which matches the energy gap between the target eigenstate |ψθ(β)> and its orthogonal counterpart |φθ(β)>.
    • Rabi Frequency Extraction: At resonance, the coherent transition probability between the two eigenstates is measured as a function of the perturbation duration (τ). This oscillation is fitted to extract the effective Rabi frequency (νe).
    • QFI Calculation: The QFI (Fβ) is calculated directly from the measured νe, the modulation amplitude (aβ), and the modulation frequency (ω) using the relation Fβ = 4(νe / (aβω))2.
  5. Phase Estimation and QCRB Verification:

    • An inverse evolution sequence (Yπ followed by Yπ-θ) is applied to rotate the final state back to the computational basis.
    • Projective measurements (Pα) are performed by counting spin-dependent fluorescence photons accumulated over many sweeps.
    • The optimal measurement sensitivity (δβ) is determined by maximizing the signal slope (χα) and minimizing the uncertainty (Δp), confirming that the measured sensitivity saturates the QCRB (δβ proportional to 1/sqrt(Fβ)).

The demonstrated technology, rooted in solid-state quantum metrology using NV centers, has direct relevance across several high-tech sectors.

Industry/SectorApplication/Product RelevanceTechnical Benefit
Quantum Metrology & SensingHigh-precision magnetometers, electrometers, and inertial sensors (gyroscopes) based on solid-state qubits.Enables rigorous, independent verification that a quantum sensor is operating at its fundamental theoretical limit (QCRB), ensuring maximum achievable precision.
Quantum Computing HardwareCharacterization and benchmarking of multi-qubit registers (e.g., NV-nuclear spin systems).Provides a scalable, non-tomographic method to quantify entanglement and information content (QFI) in complex quantum states, crucial for quality control and optimization of quantum processors.
Nanoscale Materials CharacterizationScanning probe microscopy and magnetic resonance imaging (MRI) using single NV centers.Optimizes the measurement protocol to achieve the highest possible spatial resolution and sensitivity for detecting individual spins or magnetic fields in materials.
Quantum Control SystemsDevelopment and validation of optimal control sequences for quantum systems.The QFI measurement serves as a robust, experimental figure of merit for assessing the efficiency of resource state preparation and control pulses in real-world devices.
Fundamental Physics ResearchExperimental exploration of quantum speed limits and quantum geometry in condensed matter systems.Offers a universal tool to probe geometric properties of quantum states, independent of specific estimation tasks.