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High aspect ratio diamond nanosecond laser machining

MetadataDetails
Publication Date2023-06-15
JournalApplied Physics A
AuthorsNatalie C. Golota, David Preiss, Zachary P. Fredin, Prashant Patil, Daniel Banks
InstitutionsMIT-Harvard Center for Ultracold Atoms, Massachusetts Institute of Technology
Citations16
AnalysisFull AI Review Included

This research demonstrates advanced nanosecond (ns) laser machining techniques for fabricating high aspect ratio (AR) structures in Type Ib HPHT diamond, focusing on maximizing AR and minimizing laser-induced damage.

  • Maximum Aspect Ratio Achieved: A maximum AR of 66:1 (with an average of ~40:1) was achieved using rotary assisted drilling combined with high pulse accumulation (> 1.68 M equivalent pulses).
  • Precision Taper Control: Low-taper 10:1 AR tubes were fabricated with a minimum internal taper angle of 0.11°, significantly below the Gaussian beam divergence angle (1.38°).
  • Ablation Regimes: Two distinct ablation regimes were identified during percussion drilling: Gentle (low fluence, subject to incubation effects) and Strong (high fluence, resulting in greater hole diameter eccentricity).
  • Damage Characterization: High-energy ns laser irradiation induced significant internal tensile strain, increasing up to 36% (48-55.4 MPa) in the crystal lattice, confirmed via confocal Raman spectroscopy.
  • Strain Mitigation: The laser-induced strain was successfully reduced by up to ~50% and homogenized across the sample following a 24-hour heat treatment at 600 °C in air.
  • Method Accessibility: The results were achieved using a commercially available ns laser system, providing an accessible method for fabricating high-performance diamond microstructures.
ParameterValueUnitContext
Laser Wavelength532nmDiode-pumped Nd:YAG system
Pulse Duration~20nsQ-switched operation
Repetition Rate5kHzFixed operating frequency
Maximum Average Power2.97WSystem limit
Max Aspect Ratio (Rotary Drilling)66:1 (Avg 40:1)1:1Achieved with > 1.68 M equivalent pulses
Max Aspect Ratio (Percussion Drilling)22.4 ± 1.81:1Achieved with 10,000 pulses at 177 ”J
Minimum Internal Taper Angle0.11-0.17°Taper excluding chamfer in 10:1 AR tubes
Gentle Ablation Threshold Fluence (10,000 pulses)12.4 ± 1.4J/cm2Ablation threshold decreases with pulse number
Single Pulse Ablation Threshold Fluence29.5 ± 1.3J/cm2Highest threshold observed
Incubation Coefficient0.919 ± 0.008N/AObserved in gentle ablation regime
Maximum Induced Tensile Strain55.4MPaObserved after 592 ”J finishing passes
Strain Reduction Post-Treatment~50%Reduction of laser-induced strain after annealing
Heat Treatment Parameters600°C24 h duration in air (atmospheric pressure)
Raman Shift/Strain Conversion360MPa/cm-1Linear relationship used for strain mapping
  1. Material Selection: Used Type Ib HPHT single crystal diamond with four-point 100 crystal orientation.
  2. Percussion Hole Drilling: Performed using single pulse energies ranging from 6.8 to 594 ”J. Hole geometry was characterized using microCT (2.1 ”m voxel size) to define Gentle and Strong ablation regimes.
  3. Rotary Assisted Drilling (High AR): Employed a custom apparatus using a direct drive rotary stage (66.6 RPM). High AR was achieved by translating the diamond stock while maintaining laser position and negatively incrementing the focus into the material (up to 250 ”m depth increments).
  4. Low Taper Tube Drilling (10:1 AR): Inner diameter taper was minimized by varying the irradiation profile, specifically using ramped pulse energy during initial rough cuts and final finishing passes. This technique optimizes debris and vapor ejection dynamics to reduce beam attenuation.
  5. Chamfer Control: The entrance chamfer (a 100-200 ”m deep feature) was found to be positively correlated with single pulse energy, requiring careful control or subsequent removal if detrimental.
  6. Strain Mapping: Confocal Raman spectroscopy (532 nm, 15 mW power) was used on cross-sectioned samples to map internal strain distribution and confirm the presence of surface localized sp2 carbon (graphite/amorphous carbon).
  7. Post-Processing Annealing: Oxidative heat treatment was applied at 600 °C for 24 hours in ambient air to remove surface graphite and relieve non-equilibrium bond distances, resulting in strain homogenization and reduction.

The ability to machine high-precision, low-taper, high-AR structures in diamond using accessible nanosecond lasers supports several advanced technological fields:

  • Nuclear Magnetic Resonance (NMR): Fabrication of ultra-low taper diamond sample holding tubes (rotors) required for high-speed pneumatic rotation (> 7 x 106 RPM) in MAS NMR research.
  • Quantum Technology: Manufacturing microstructures for next-generation quantum devices, including those based on nitrogen-vacancy (NV) centers, where precise geometry and minimal lattice strain are critical.
  • Micro-Electromechanical Systems (MEMS): Production of high-strength diamond components for MEMS devices, leveraging diamond’s superior mechanical properties.
  • Microfluidics and Sensing: Creation of biocompatible microfluidic channels and spectroscopic devices, benefiting from diamond’s chemical inertness and optical transparency.
  • High-Power Electronics: Fabrication of thermally optimized microstructures for power electronics and heat sinks, utilizing diamond’s exceptional thermal conductivity.