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Maser threshold characterization by resonator Q-factor tuning

MetadataDetails
Publication Date2023-10-14
JournalCommunications Physics
AuthorsChristoph W. Zollitsch, Stefan Ruloff, Yan Fett, Haakon T. A. Wiedemann, Rudolf Richter
InstitutionsLondon Centre for Nanotechnology, University College London
Citations9
AnalysisFull AI Review Included

This research details the design and characterization of an optimized continuous-wave (CW) room-temperature maser utilizing Nitrogen-Vacancy (NV-) centers in diamond.

  • Core Achievement: The study experimentally verified the maser threshold equation over a wide parameter space by systematically tuning the loaded quality factor (QL) of the microwave resonator and the optical pump rate (wL), which controls spin level-inversion.
  • Performance Benchmark: The optimized setup achieved a maximal CW maser output power of -54.1 dBm, representing an improvement of more than three orders of magnitude compared to previous NV- maser reports (-90.3 dBm).
  • Optimal Operation Regime: Continuous masing was found to be most efficient in the highly under-coupled regime (high QL), where intrinsic resonator losses dominate external coupling losses.
  • Threshold Identification: The maser threshold diagram clearly identified the minimal requirements for continuous emission, requiring QL > 26,000 and wL > 200 s-1 for stable operation.
  • Thermal Management Importance: Laser pumping caused significant heating, reducing the spin longitudinal relaxation time (T1) from 5.2 ms (low pump) to 1.5 ms (high pump), highlighting thermal management as critical for maximizing spin inversion and limiting the masing threshold.
  • Engineering Blueprint: The work provides a quantitative blueprint for future solid-state maser systems, focusing on maximizing Qint to enable higher output coupling while maintaining stable operation.
ParameterValueUnitContext
Maser MaterialNV- centers in diamond0.16 ppmNatural abundance carbon
Operation TemperatureRoom TemperatureN/AContinuous-Wave (CW)
Resonance Frequency (ωres/2π)9.12GHzX-band, TE018 mode
Resonator MaterialSapphire RingN/AHoused in Ag/Au plated Copper cavity
Loaded Q-Factor (QL) Range14,000 to 33,500N/ATuned via coupling screw
Unloaded Internal Q-Factor (Qint)42,500N/AFully under-coupled, without sample
Critical Coupling (k=1) QL~20,000N/ATransition point
Maximum Maser Output Power-54.1dBmAchieved at highest QL and wL
Laser Pump Wavelength532nmUsed for optical spin polarization
Laser Pump Rate (wL) Range165 to 695s-1Controls level-inversion
Maser Threshold QL>26,000N/ARequired for continuous masing
Spin Relaxation Time (T1)5.2 to 1.5msDecreases with increasing laser heating
Spin Coherence Time (T2)25”sMeasured via pulsed ESR (no pump)
Total NV- Spins (N)2.32 x 1013N/APer hyperfine transition/defect axis
  1. Cavity and Resonator Construction: A cylindrical cavity made of oxygen-free high-thermal conductivity copper, plated with silver and gold to minimize resistive losses, was designed to fit between electromagnet poles. A sapphire dielectric ring resonator was placed centrally, operating in the TE018 mode (9-10 GHz).
  2. Q-Factor Tuning Mechanism: The external quality factor (Qext) was controlled via a single waveguide iris port. A Teflon screw tipped with a metal ring adjusted the iris coverage, allowing continuous tuning of the loaded quality factor (QL) from over-coupled (low QL) to fully under-coupled (high QL).
  3. NV- Alignment and Characterization: The diamond sample, held in a quartz tube, was rotated using a goniometer relative to the static magnetic field (B0). Conventional Electron Spin Resonance (ESR) spectroscopy was used to align the NV- defect axis parallel to B0, maximizing the Zeeman splitting and initial Boltzmann population difference.
  4. Spin Inversion Control: A 532 nm laser was used for continuous optical pumping. The laser power was systematically varied to control the pump rate (wL) and, consequently, the degree of spin level-inversion (η), which is a key factor in the maser threshold equation.
  5. Maser Threshold Mapping: The peak maser emission power (|AM|) was measured using a spectrum analyzer preceded by a low-noise amplifier (LNA). Measurements were performed across the full range of tunable QL and wL, generating a comprehensive maser threshold diagram.
  6. System Parameter Extraction: System parameters (e.g., T1, N, Îł, g0) required for theoretical modeling (Tavis-Cummings model) were determined via low-power microwave spectroscopy and finite element simulations, including explicit measurement of T1 reduction due to laser heating.

The successful optimization and characterization of a room-temperature, high-power CW maser based on NV- diamond opens pathways for several advanced engineering applications:

  • Ultra-Low-Noise Amplification:
    • Deployment in deep-space antenna networks and radio astronomy where extremely low-noise microwave amplification is critical, traditionally requiring bulky cryogenic systems.
    • High-fidelity signal amplification in sensitive detection systems (e.g., magnetic resonance imaging or quantum computing readout).
  • Enhanced Quantum Sensing:
    • Use as a high-gain, low-noise amplifier to boost the signal-to-noise ratio (SNR) in room-temperature quantum sensors utilizing molecular spin ensembles.
  • Microwave Frequency Standards:
    • Development of compact, room-temperature frequency standards leveraging the stable maser emission frequency.
  • Solid-State Device Engineering:
    • The optimized setup serves as a validated testbed and blueprint for characterizing and optimizing masers based on other solid-state materials (e.g., Silicon Carbide, SiC), accelerating the development of next-generation microwave devices.
  • Integrated Microwave Platforms:
    • Establishing maser technology as a viable, non-cryogenic platform for general microwave research and development, enabling miniaturization and integration into commercial systems.
View Original Abstract

Abstract Whereas the laser is nowadays an ubiquitous technology, applications for its microwave analog, the maser, remain highly specialized, despite the excellent low-noise microwave amplification properties. The widespread application of masers is typically limited by the need of cryogenic temperatures. The recent realization of a continuous-wave room-temperature maser, using NV − centers in diamond, is a first step towards establishing the maser as a potential platform for microwave research and development, yet its design is far from optimal. Here, we design and construct an optimized setup able to characterize the operating space of a maser using NV − centers. We focus on the interplay of two key parameters for emission of microwave photons: the quality factor of the microwave resonator and the degree of spin level-inversion. We characterize the performance of the maser as a function of these two parameters, identifying the parameter space of operation and highlighting the requirements for maximal continuous microwave emission.