Skip to content

Measurement of Neutrons Produced by Inertial Fusion with a Diamond Radiation Detector

MetadataDetails
Publication Date2024-01-25
JournalSensors and Materials
AuthorsTakehiro Shimaoka, Junichi H. Kaneko, Yasunobu Arikawa, Masakatsu Tsubota Mitsutaka Isobe, Kengo Oda
InstitutionsNational Institute of Advanced Industrial Science and Technology, The University of Osaka
Citations1
AnalysisFull AI Review Included

This research validates the use of single-crystal Chemical Vapor Deposition (CVD) diamond detectors for critical diagnostics in Inertial Confinement Fusion (ICF) experiments.

  • Breakthrough Detection: Successful first-time observation of Deuterium-Deuterium (DD) neutron signals using a single-crystal CVD diamond detector at fluences of 108 neutrons/shot or higher.
  • Noise Mitigation: The measurement system employed extensive electromagnetic shielding, electrical floating (using UPS battery power), and optical fiber triggering to overcome strong electromagnetic noise generated by laser irradiation.
  • Material Advantage: Single-crystal diamond offers superior charge collection efficiency and, crucially, exhibits no afterpulse or afterglow, solving major limitations faced by plastic scintillators under intense bremsstrahlung X-ray backgrounds (1012-1015 photons/shot).
  • Application Validation: The detector’s fast response successfully discriminated between X-ray and DD neutron signals (6.2 ns time difference), confirming its suitability for neutron Time-of-Flight (ToF) measurements.
  • Future Potential: The detector is expected to be effective for measuring neutron bang time and burn history in future fast ignition experiments (FIREX), where neutron yields are projected to reach 1011 neutrons/shot.
  • Performance: The detector demonstrated a charge collection efficiency of nearly 100% for both electrons and holes, ensuring high reliability in yield evaluation.
ParameterValueUnitContext
Detector MaterialSingle-crystal CVD DiamondN/AHomoepitaxially grown
Detector Area5 x 5mm2Freestanding film size
Detector Thickness150”mFreestanding film thickness
Schottky ElectrodeAl (3.0 mm diameter, 100 nm thick)N/AFabricated on as-grown surface
Ohmic ElectrodeTiC/Au (3.0 mm diameter, 100 nm thick)N/AFabricated on substrate side
Charge Collection EfficiencyAlmost 100%For both electrons and holes
Required Time ResolutionBetter than 100psFor bang time measurement
Required Detector DistanceWithin 5.7cmTo achieve 100 ps resolution at 5 keV Ti
Actual Detector Distance14.5cmUsed in GEKKO XII experiment
Neutron Yield Detected108neutrons/shotMinimum yield successfully measured
Expected FIREX Yield1011neutrons/shotExpected yield for successful fast ignition
Neutron Sensitivity2 x 10-8mV/neutronWave height sensitivity for DD neutrons
Expected Output Signal (1011 n/shot)2VBased on linear scaling of sensitivity
Electromagnetic Noise Level2mV peak-to-peakAchieved noise level during measurement
X-ray / DD Neutron Time Difference6.2nsCorresponds to 14.5 cm distance
DD Neutron Energy2.45MeVProduced by DD reaction

The experiment focused on high-quality sample preparation and rigorous noise mitigation techniques to enable Time-of-Flight (ToF) measurement of DD neutrons generated by the GEKKO XII laser.

  1. Sample Preparation (CVD Growth):

    • Substrate: HP/HT IIa-type substrate with off-angle control.
    • Growth Method: Microwave Plasma CVD (System 5250; ASTEX).
    • Growth Conditions: Gas pressure of 110 Torr, substrate temperature of 850 °C, microwave power of 1000 W.
    • Gas Mixture: CH4/[H2+CH4] concentration of 0.25%.
    • Lift-Off: The grown layer was separated by electrolytic etching to obtain a freestanding film (150 ”m thick).
  2. Detector Fabrication and Characterization:

    • Electrodes: Al Schottky electrode (100 nm thick) deposited on the as-grown surface; TiC/Au Ohmic electrode (100 nm thick) deposited on the substrate side.
    • Efficiency Check: Charge collection efficiency was confirmed to be almost 100% using alpha-ray-induced charge distribution measurement.
  3. Noise Reduction and Electrical Floating:

    • Shielding: The detector, coaxial cable, and measurement instruments were installed in a metal GS tube and a laboratory-made Cu shielded box.
    • Isolation: The detector port was insulated from the target chamber using an acrylic flange. The entire system was electrically floated using UPS battery power to drive instruments.
    • Triggering: The trigger signal was transmitted via an optical fiber and photodiode to eliminate electrical noise coupling.
  4. Neutron Measurement (GEKKO XII):

    • Target: Thin 2-3 ”m thick deuterium-gas-filled CD shells were used to maximize neutron generation (108 neutrons/shot).
    • Instrumentation: Bias tee (16 GHz bandwidth), oscilloscope (4 GHz bandwidth, 20 GS/s sampling rate) were used for high-speed signal acquisition.
    • Confirmation: Neutron signals were confirmed by comparing the output pulse wave height at the expected arrival time (-37 ns) with shots using deuterium-free CH shells (which showed no signal).

The development of high-speed, radiation-hard single-crystal diamond detectors is critical for applications requiring diagnostics in extreme environments characterized by high neutron flux and intense X-ray backgrounds.

  • Fusion Energy Research:
    • Neutron bang time and burn history monitoring in ICF facilities (e.g., NIF, GEKKO XII, FIREX).
    • Plasma diagnostics requiring high time resolution (less than 100 ps) under intense X-ray loads.
  • High-Energy Physics and Accelerators:
    • Beam monitoring and dosimetry in high-flux particle accelerators where radiation damage is a concern.
    • Time-resolved detection of nuclear reaction products.
  • Nuclear Security and Safeguards:
    • Fast, radiation-hard neutron detection systems for monitoring nuclear materials and processes.
  • High-Power Electronics (Indirectly Related):
    • The underlying single-crystal CVD growth technology is essential for producing high-quality diamond substrates used in high-power, high-frequency electronic devices (e.g., 6ccvd.com products like thermal management materials and high-voltage switches).
  • Extreme Environment Sensing:
    • Sensors operating in environments with high temperatures and intense radiation fields where conventional semiconductor materials fail.
View Original Abstract

We evaluated the neutron bang time in fast-ignition inertial confinement fusion and the response function of deuterium-deuterium (DD) neutrons for burn history monitoring applications with a single-crystal CVD diamond detector.Signals were successfully obtained for the first time with a single-crystal diamond detector for DD neutrons of above 10 8 neutrons/shot.