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Wurtzite silicon as a potential absorber in photovoltaics - Tailoring the optical absorption by applying strain

MetadataDetails
Publication Date2015-07-20
JournalPhysical Review B
AuthorsClaudia Rödl, Tobias Sander, F. Bechstedt, Julien Vidal, PÀr Olsson
InstitutionsCentre National de la Recherche Scientifique, Friedrich Schiller University Jena
Citations71

We present ab initio calculations of the electronic structure and the optical properties of wurtzite Si (Si-IV). We find an indirect band gap of 0.95 eV $({\mathrm{\ensuremath{\Gamma}}}{5}\ensuremath{\rightarrow}{M}{1})$ and an optically forbidden direct gap of 1.63 eV $({\mathrm{\ensuremath{\Gamma}}}{5}\ensuremath{\rightarrow}{\mathrm{\ensuremath{\Gamma}}}{10})$, which is due to a backfolding of the ${L}_{1}$ state of Si in the diamond structure (Si-I). Optical absorption spectra including excitonic and local-field effects are calculated. Further, the effects of hydrostatic pressure, uniaxial strain, and biaxial strain on the absorption properties are investigated. Biaxial tensile strains enhance the optical absorption of Si-IV in the spectral range which is relevant for photovoltaic applications. High biaxial tensile strains $(>4%)$ even transform Si-IV into a direct semiconductor.