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Mapping Dynamical Magnetic Responses of Ultrathin Micron-Size Superconducting Films Using Nitrogen-Vacancy Centers in Diamond

MetadataDetails
Publication Date2019-07-26
JournalNano Letters
AuthorsYing Xu, Yijun Yu, Yuen Yung Hui, Yudan Su, Jun Cheng
InstitutionsState Key Laboratory of Surface Physics, University of California, Berkeley
Citations22

Two-dimensional superconductors have attracted growing interest because of their scientific novelty, structural tunability, and useful properties. Studies of their magnetic responses, however, are often hampered by difficulties to grow large-size samples of high quality and uniformity. We report here an imaging method that employed NV<sup>-</sup> centers in diamond as a sensor capable of mapping out the microwave magnetic field distribution on an ultrathin superconducting film of micron size. Measurements on a 33 nm thick film and a 125 nm thick bulklike film of Bi<sub>2</sub>Sr<sub>2</sub>CaCu<sub>2</sub>O<sub>8+Γ</sub> revealed that the alternating current (ac) Meissner effect (or repulsion of ac magnetic field) set in at 78 and 91 K, respectively; the latter was the superconducting transition temperature of both films. The unusual ac magnetic response of the thin film presumably was due to thermally excited vortex-antivortex diffusive motion in the film. Spatial resolution of our ac magnetometer was limited by optical diffraction and the noise level was at 14 μT/Hz<sup>1/2</sup>. The technique could be extended with better detection sensitivity to extract local ac conductivity/susceptibility of ultrathin or monolayer superconducting samples as well as ac magnetic responses of other two-dimensional exotic thin films of limited lateral size.