Skip to content

Strong polarization of individual nuclear spins weakly coupled to nitrogen-vacancy color centers in diamond

MetadataDetails
Publication Date2019-09-01
JournalNew Journal of Physics
AuthorsJiwon Yun, Kiho Kim, Dohun Kim, Jiwon Yun, Kiho Kim
InstitutionsSeoul National University
Citations7

Abstract We experimentally demonstrate high degree of polarization of 13 C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled relaxation and achieve a polarity-tunable, fast nuclear polarization of degree higher than 85% at room temperature for remote 13 C nuclear spins exhibiting hyperfine interaction strength with NV centers of the order of 600 kHz. We show with the aid of numerical simulation that the anisotropic hyperfine tensor components naturally provide a route to control spin mixing parameter so that highly efficient nuclear polarization is enabled through careful tuning of nuclear quantization axis by external magnetic field. We further discuss spin dynamics and wide applicability of this method to various target 13 C nuclear spins around the NV center electron spin. The proposed control method demonstrates an efficient and versatile route to realize, for example, high-fidelity spin register initialization and quantum metrology using nuclear spin resources in solids.

  1. 1998 - A silicon-based nuclear spin quantum computer [Crossref]
  2. 2012 - Room-temperature quantum bit memory exceeding one second [Crossref]
  3. 2014 - Storing quantum information for 30 s in a nanoelectronic device [Crossref]
  4. 2014 - Coherent control of a single 29Si nuclear spin qubit [Crossref]
  5. 1997 - Scanning confocal optical microscopy and magnetic resonance on single defect centers [Crossref]
  6. 1946 - Resonance absorption by nuclear magnetic moments in a solid [Crossref]
  7. 2017 - Arbitrary nuclear-spin gates in diamond mediated by a nitrogen-vacancy-center electron spin [Crossref]
  8. 2016 - Robust quantum-network memory using decoherence-protected subspaces of nuclear spins [Crossref]
  9. 2009 - Dynamic polarization of single nuclear spins by optical pumping of nitrogen-vacancy color centers in diamond at room temperature [Crossref]
  10. 2015 - Strongly polarizing weakly coupled 13C nuclear spins with optically pumped nitrogen-vacancy center [Crossref]