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Focusing the electromagnetic field to 10−6λ for ultra-high enhancement of field-matter interaction

MetadataDetails
Publication Date2021-11-04
JournalNature Communications
AuthorsXiang-Dong Chen, Enhui Wang, Long‐Kun Shan, Ce Feng, Y. H. Zheng
InstitutionsUniversity of Science and Technology of China
Citations28
AnalysisFull AI Review Included
  • Core Achievement: Demonstrated ultra-tight localization of microwave electromagnetic fields down to 291 nm, corresponding to a deep-subwavelength scale of 10-6λ.
  • Mechanism: Achieved localization via direct coupling with confined electron oscillations in a low-dimensional Ag nanowire, utilizing near-field radiation governed by the Biot-Savart law.
  • Performance Metric (Intensity): Realized an unprecedented local microwave field intensity enhancement of 2.0 x 108 times compared to far-field excitation.
  • Performance Metric (Interaction): Enhanced the microwave-spin interaction strength (Rabi oscillation frequency) by 1.4 x 104 times, enabling fast spin qubit manipulation.
  • Device Structure: A hybrid nanowire-bowtie antenna designed to focus free-space microwave signals directly into the deep-subwavelength volume.
  • Detection Method: Used Nitrogen Vacancy (NV) centers in diamond as a non-invasive quantum probe, mapped with high spatial resolution (~100 nm) using Charge State Depletion (CSD) nanoscopy.
  • Future Impact: This high concentration of microwave field is critical for promoting integrated quantum information processing, nanoscale sensing, and microwave photonics systems.
ParameterValueUnitContext
Field Localization Scale2.8 x 10-6λ (291 ± 10)Dimensionless (nm)Width of the microwave magnetic component cross-section profile
Field Intensity Enhancement2.0 x 108TimesIncrease in local microwave intensity compared to far-field
Rabi Frequency Enhancement1.4 x 104TimesIncrease in microwave-spin interaction strength
Microwave Wavelength (λ)10.4cmCorresponding to 2.87 GHz resonant frequency in vacuum
Ag Nanowire Diameter120nmDiameter of the low-dimensional conductor
Bowtie Antenna Gap (Wgap)8µmDistance between the two metallic arms
Bowtie Antenna Length6.5cmOverall length of the metallic structure
NV Center Depth~20nmDepth of the NV centers below the diamond surface
NV Center Resonant Frequency2.87GHzSpin transition frequency (ms = 0 to ms = ±1)
CSD Nanoscopy Resolution~100nmSpatial resolution used for ODMR mapping
Enhanced Rabi Frequency1.6µs-1Measured under the nanowire-bowtie antenna (PMW = 14 µW)
  1. Sample Preparation (NV Centers): Electrical grade diamond plates ({100} surface) were implanted with nitrogen ions (15 keV energy, 1013/cm2 dosage) and subsequently annealed at 850 °C for 2 hours to generate NV center ensembles (~5000/µm2 density).
  2. Hybrid Antenna Fabrication: A metallic bowtie structure (5 nm Chromium / 200 nm Gold film) was patterned onto the diamond surface using lift-off. An Ag nanowire (120 nm diameter) was then deposited via spin processing to complete the hybrid structure.
  3. Microwave Excitation: Far-field microwave signals were generated by two microwave generators, combined, amplified, and radiated into free space using a double-ridged horn antenna positioned approximately 20 cm from the device.
  4. Optical Detection System: A home-built confocal microscope was used for Optically Detected Magnetic Resonance (ODMR) measurements. Lasers (532 nm, 589 nm, 637 nm) were modulated by acousto-optic modulators (AOMs).
  5. High-Resolution Mapping (CSD Nanoscopy): The localized microwave field distribution was mapped using Charge State Depletion (CSD) nanoscopy, which achieves diffraction-unlimited resolution (~100 nm) by manipulating and detecting the NV center charge state.
  6. Interaction Strength Quantification: The enhancement of the microwave-spin interaction was quantified by measuring the Rabi oscillation frequency (in µs-1) of the NV centers under continuous-wave microwave pumping for various antenna configurations.

The technology, based on ultra-high electromagnetic field concentration and efficient spin manipulation, is relevant to the following fields:

  • Quantum Information Processing (QIP): Enables individual addressing and fast coherent manipulation of multi-qubits (e.g., trapped ions or solid-state spins) using highly localized microwave gradients.
  • Nanoscale Quantum Sensing: Promotes the development of ultra-weak microwave signal sensing (e.g., quantum radar) and high-sensitivity spin-based metrology by increasing the signal-to-noise ratio by 104 times.
  • Integrated Microwave Photonics: Provides a platform for delivering and concentrating both light (via the Ag nanowire’s light-guiding effect) and microwave fields, facilitating miniaturized, integrated quantum devices.
  • Cryogenic Electronics: Simplifies quantum processing devices by enabling efficient far-field pumping, potentially reducing Johnson noise and thermal leakage associated with large metal films near qubits in cryostats.
  • Hybrid Quantum Systems: Offers a solution for efficient coupling between microwave circuits and optical components (like NV center fluorescence collection) in a compact, wireless platform.