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Combination of granular activated carbon adsorption and electrochemical oxidation processes in methanol medium for benzene removal

MetadataDetails
Publication Date2022-06-05
JournalElectrochimica Acta
AuthorsRodrigo de Mello, Artur de Jesus Motheo, Cristina SƔez, Manuel A. Rodrigo
InstitutionsUniversity of Castilla-La Mancha, Universidade Federal de SĆ£o Carlos
Citations15

One of the impacts caused by the increase in anthropogenic activities, related to the accelerated urbanization and industrialization, is the increase in emissions of volatile organic compounds (VOC). This type of air pollution has become a matter of great concern nowadays, because of its harmfulness to the environment and human health. Adsorption technologies are one of the most promising methods for decontaminating VOCs from the air because they are simple, inexpensive, and energy efficient. On the other hand, electrochemical treatments have been extensively and successfully studied for water treatment. The combination of an adsorption step followed by an electrochemical treatment, with the regeneration of the adsorbent material, can be an interesting alternative, mainly to overcome the limitations of the treatment of diluted solutions. In this work, the removal of benzene from diluted water solutions were evaluated using a combination of three processes: adsorption, desorption with methanol and electrochemical oxidation with boron-doped diamond electrode (BDD) of the high concentrated solution obtained. This technology is suitable for the recovery of the adsorbent material (granular activated carbon), which can be reused after drying. Two possible concurrent ways to remove benzene from methanol solutions by electrochemical oxidation were found: (1) mineralization and (2) conversion to anisole, a solvent of commercial interest used in the cosmetics industry. The performance of electrochemical treatment for benzene removal from methanol solution was not so different than that in water, but the energy consumption was greater. However, the production of high added-value products is a very interesting finding that will advance the development of more sustainable treatment processes.

  1. 2015 - Coal combustion and the environment
  2. 2019 - Recent advancements in photocatalyst-based platforms for the destruction of gaseous benzene: Performance evaluation of different modes of photocatalytic operations and against adsorption techniques [Crossref]
  3. 2018 - Enhanced photocatalytic decomposition of VOCs by visible-driven photocatalyst combined Cu-TiO2 and activated carbon fiber [Crossref]
  4. 2020 - A critical review on VOCs adsorption by different porous materials: species, mechanisms and modification methods
  5. 2018 - Regeneration of activated carbon fiber by the electro-fenton process [Crossref]
  6. 2020 - Evaluation of electrolytic reactor configuration for the regeneration of granular activated carbon saturated with methylene blue [Crossref]
  7. 2018 - Alachlor removal performance of Ti/Ru0.3Ti0.7O2 anodes prepared from ionic liquid solution [Crossref]
  8. 2018 - Indirect electrochemical oxidation of 2,4-dichlorophenoxyacetic acid using electrochemically-generated persulfate [Crossref]