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Super-Resolution Airy Disk Microscopy of Individual Color Centers in Diamond

MetadataDetails
Publication Date2022-08-31
JournalACS Photonics
AuthorsAedan Gardill, Ishita Kemeny, Yanfei Li, Maryam Zahedian, Matthew Carl Cambria
InstitutionsLawrence Livermore National Laboratory, HUN-REN Wigner Research Centre for Physics
Citations15

Super-resolution imaging techniques enable nanoscale microscopy in fields such as physics, biology, and chemistry. However, many super-resolution techniques require specialized optical components, such as a helical-phase mask. In this work, we present a novel technique, super-resolution Airy disk microscopy, that can be used in a standard confocal microscope without any specialized optics. We demonstrate this technique, in combination with ground state depletion, to image and control nitrogen-vacancy (NV) centers in bulk diamond below the diffraction limit. A greater than 14-fold improvement in resolution compared to the diffraction limit is achieved, corresponding to a spatial resolution of 16.9(8) nm for a 1.3 NA microscope with 589 nm light. We make use of our enhanced spatial resolution to control the spins states of individual NV centers separated from each other by less than the diffraction limit, including pairs sharing the same orientation that are indistinguishable with a conventional electron spin resonance measurement.