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Nitrogen-Vacancy Singlet-Manifold Ionization Energy

MetadataDetails
Publication Date2023-03-23
JournalPhysical Review Applied
AuthorsS. A. Wolf, Idan Meirzada, Galya Haim, Nir Bar‐Gill
InstitutionsHebrew University of Jerusalem, The University of Melbourne
Citations6

<p>Abstract:</p> <p>The singlet states of the negatively charged nitrogen-vacancy centers in diamond play a key role in its<br>optical spin control and readout. In this work, the hitherto unknown ionization energy of the singlet is<br>measured experimentally and found to be in the range 1.91–2.25 eV. This is obtained by analyzing photo-<br>luminescence measurements incorporating spin control and nitrogen-vacancy charge state differentiation,<br>along with simulations based on the nitrogen-vacancy’s master equation. This work establishes a proto-<br>col for a more accurate estimate of this ionization energy, which can possibly lead to improved readout<br>methods.</p>