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Ultrastrong magnetic light-matter interaction with cavity mode engineering

MetadataDetails
Publication Date2023-05-18
JournalCommunications Physics
AuthorsHyeongrak Choi, Dirk Englund
Citations2
AnalysisFull AI Review Included

This research details novel mode engineering techniques for hollow metallic cavities to achieve unprecedentedly strong magnetic light-matter interaction, crucial for quantum technologies.

  • Ultrastrong Coupling Achieved: The magnetic interaction figure of merit (Q/VB) was enhanced by more than 1016 times compared to free space, representing an improvement of five orders of magnitude over existing cavity designs.
  • Arbitrarily Small Mode Volume: The effective magnetic mode volume (VB) can be reduced arbitrarily, limited only by the material’s electromagnetic penetration depth (e.g., 40 nm for Niobium).
  • Three Core Methods: VB reduction is achieved via (1) Longitudinal Mode Squeezing, (2) Current Engineering (using inverse-tapered reentrances for current crowding), and (3) Magnetic Field Expulsion (using thin metallic plates).
  • Superconducting Advantage: Utilizing superconducting materials (Niobium) allows for ultrahigh quality factors (Q > 109) by minimizing ohmic losses, enabling the maximum Q/VB ratio.
  • Experimental Validation: Proof-of-principle experiments using diamond Nitrogen-Vacancy (NV) spin ensembles confirmed the theoretical predictions for VB, Q, and resonance frequency (f ā‰ˆ 2.87 GHz).
  • Enabling Technology: These methods pave the way for high-cooperativity microwave-spin coupling, compact Electron Paramagnetic Resonance (EPR) sensors, and fundamental science applications like dark matter searches.
ParameterValueUnitContext
Maximum Q/VB (Theoretical)3 x 1016λ-3Combined current engineering and field expulsion (Niobium, 1 µm plate)
Maximum Q (Theoretical)1.06 x 109N/AAchieved using Niobium (Rs = 10 nΩ)
Minimum VB (Theoretical)3.6 x 10-9λ3Achieved using Niobium (Rs = 10 nΩ)
Niobium (Nb) Surface Resistance (Rs)1 - 10nΩSuperconducting material loss (T < 4.2 K)
Copper (Cu) Surface Resistance (Rs)1mΩNormal conductor loss (at 1 K)
Niobium London Penetration Depth (λL)40nmUltimate limit for VB reduction
Copper Skin Depth (1 GHz)2µmLimit for VB reduction in normal conductors
Experimental VB (Doubly Reentrant)1.75 x 10-3λ3Measured using NV centers (f = 2.929 MHz Rabi frequency)
Experimental Q (Doubly Reentrant)2,421N/AMeasured at f = 2.871 GHz (Copper cavity)
NV Center Coherence Time (T2)Up to 1.5msRoom temperature diamond
Calculated Single-Spin Cooperativity (C)12.5N/ASingle NV center at 10 GHz, VB = 3.62 x 10-8 λ3
Sapphire Dielectric Loss (Qdielectric)1.45 x 1010N/AEstimated additional loss from substrate in field-expulsion cavity

The study employed three primary methods, often combined, to manipulate the electromagnetic fields within hollow metallic cavities, focusing on the Transverse Magnetic (TM) modes.

  1. Longitudinal Mode Squeezing (TM010 Mode):

    • Principle: The TM010 mode’s resonant frequency is independent of the cavity height (h).
    • Implementation: Decreasing h (longitudinal squeezing) reduces VB proportionally to h, achieving VB less than the diffraction limit (Ī»3).
    • Limitation: VB reduction is ultimately limited by the metal’s penetration depth (Ī“).
  2. Current Engineering (Reentrant Cavities):

    • Principle: Locally increasing the surface current density (Js) enhances the magnetic field (B), thereby reducing VB (VB āˆ 1/B2).
    • Designs: Framework integrates split-mode, loop-gap, and reentrant cavities.
    • Current Crowding via Inverse-Tapering: Modified reentrant cavities were designed with inverse-tapering (smaller bottom radius R’ < R) to combine large capacitance (charge storage) with a narrow conducting channel, maximizing current density and VB reduction.
  3. Magnetic Field Expulsion (Meissner Effect Analogy):

    • Principle: Good conductors and superconductors expel magnetic fields (Faraday’s law/Meissner effect), concentrating the field at sharp edges or gaps.
    • Implementation: A thin metallic plate (thickness t, down to 10 µm) was inserted into the cavity. The external field is circumvented, creating magnetic ā€œhot spotsā€ at the edges.
    • Scaling: VB was found to be linearly proportional to the plate thickness (t). Crucially, Q did not degrade when VB was reduced by thinning the plate.
  4. Numerical Simulation and Validation:

    • Simulation: All designs were modeled using the Finite Element Method (FEM) in COMSOL, ensuring mesh sizes were smaller than half the minimum feature size (e.g., plate thickness).
    • Experimental Setup: A doubly reentrant copper cavity (h = 1.9 cm) was fabricated and tested using an ensemble of 300 ppb NV centers in diamond as a magnetic field sensor.
    • Measurement: Optically Detected Magnetic Resonance (ODMR) was used to measure the Rabi oscillation frequency, which directly correlates to the single-photon magnetic field (Bs) and thus VB.

The ultrastrong magnetic light-matter interaction enabled by these engineered cavities is critical for advancing several high-tech fields:

  • Quantum Computing:
    • High-cooperativity coupling between microwave photons and solid-state spin qubits (e.g., NV centers, electron spins) or superconducting flux qubits.
    • Enabling compact, high-coherence 3D circuit Quantum Electrodynamics (cQED) architectures.
  • Quantum Networks and Transduction:
    • High-fidelity, thresholdless single MW-photon to optical photon transduction, essential for connecting quantum processors via optical fibers.
  • Sensing and Metrology:
    • Development of compact, high-sensitivity Electron Paramagnetic Resonance (EPR) sensors.
    • Low-noise, continuous-wave room-temperature masers (MW amplifiers).
    • Nuclear Magnetic Resonance (NMR) and ultra-precision metrology.
  • Fundamental Science:
    • High-sensitivity searches for fundamental particles, such as dark matter (axions), using high-Q microwave-spin coupling systems.
  • Microwave Devices:
    • Active microwave devices and magnetic nonlinear devices (e.g., Kerr blockade, nonlinear bistability) operating at high cooperativity.