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Thermal conduction in isotope diamond thin films studied by pump-probe laser reflectivity measurement

MetadataDetails
Publication Date2020-03-03
JournalJapanese Journal of Applied Physics
AuthorsHsu Kai Weng, Akira Nagakubo, Hideyuki Watanabe, Hirotsugu Ogi
InstitutionsThe University of Osaka, National Institute of Advanced Industrial Science and Technology
Citations6

We study the thermal conductivity of isotope-controlled diamond thin films between 0.001% and 99% 13C contents using an ultrafast pump-probe laser experiment. We measure the surface temperature change through the reflectivity change of the probe light pulse after heating with the pump light pulse, compare it with a theoretical calculation, and estimate the thermal conductivity. The Brillouin-oscillation appears in the reflectivity change, which is used for determining the film thickness and then removed in determining the thermal conductivity. The theoretical calculation reveals that the diamond film should be thicker than 1 μm for obtaining appropriate thermal conductivity. Our results indicate that the thermal conductivity of the 50%-13C diamond thin film is much lower than the reported value, suggesting unavailability of reported values of bulk materials for thin films and necessity for measurement for the thermal conductivity of thin films.