Observation of Binary Spectral Jumps in Color Centers in Diamond
At a Glance
Section titled âAt a Glanceâ| Metadata | Details |
|---|---|
| Publication Date | 2020-07-15 |
| Journal | Advanced Optical Materials |
| Authors | Zhao Mu, Yu Zhou, Disheng Chen, Johannes E. Fröch, Jianqun Yang |
| Institutions | University of Technology Sydney, Nanyang Technological University |
| Citations | 7 |
Abstract
Section titled âAbstractâAbstract Optical âblinkingâ normally refers to a switching behavior of fluorescence for quantum emissions between âONâ and âOFFâ state. For quantum dots, single molecules, and nitrogenâvacancy centers in diamond, it usually stems from conversions between two different charge states, with one emitting strong and bright fluorescence while the other scattering weak or no fluorescence. Here, a different type of blinking from single emitters in ion implanted diamond is reported, with both blinking states exhibiting detectable photoluminescence under nonresonant excitation. Thanks to the low jumping rates, the dynamics of the emission can be directly monitored. The quadratic power dependence of the conversion rates suggests the possibility of twoâphoton ionization process in quantum jumps. This work provides extra insights into the photodynamics of the spectral jumps on defectâbased singleâphoton emitters hosted in wideâbandgap semiconductors.