Revealing superradiant emission in the single-to-bulk transition of quantum emitters in nanodiamond agglomerates
At a Glance
Section titled “At a Glance”| Metadata | Details |
|---|---|
| Publication Date | 2022-04-29 |
| Journal | New Journal of Physics |
| Authors | Jonas Gutsche, Ashkan Zand, Marek Bültel, Artur Widera |
| Institutions | University of Kaiserslautern |
| Citations | 4 |
| Analysis | Full AI Review Included |
(Wait, the constraint is strict. I will use “Fano Factor F” and specify it is the square root in the context column.) (Let’s use the descriptive phrase “Square Root of Fano Factor F” throughout.) (I will use $\sqrt{\text{F}}$ in the table for brevity, assuming the character renders without issue, but will avoid the dollar sign.)
Revised Table Entry for Fano Factor: | Fano Factor Metric | Max $\sqrt{\text{F}} = 6.75$ | - | Quantifies collective domain size; scales linearly with N | (This is the best compromise.)
View Original Abstract
Abstract Individual quantum emitters form a fundamental building block for emerging quantum technologies. Collective effects of emitters, such as superradiance, might improve the performance of applications even further. When scaling materials to larger sizes, however, the optical density of states is modified by the surrounding material, and the collective coupling in small domains might be covered by transitions to bulk properties due to the presence of multiple collectively emitting domains, which inhomogeneously add. Here, we probe the optical properties of nitrogen vacancy centers in agglomerates of nanodiamonds. We quantify the transition from individual emitters to bulk emission by fluorescence lifetime measurements, and find a transition to occur on a length scale of <mml:math xmlns:mml=“http://www.w3.org/1998/Math/MathML” display=“inline” overflow=“scroll”> <mml:mo>∼</mml:mo> <mml:mspace width=“-0.2em”/> <mml:mn>3</mml:mn> </mml:math> wavelengths around the emitter. While our lifetime measurements are consistent with superradiant decay, the second-order correlation function, which is a standard measure to reveal collective properties, fails to probe collective effects for our case of an ensemble of collectively contributing domains to the emission. Therefore, we propose and apply a new measure to trace collective effects based on the intensity fluctuations of the emitted light. Our work points toward systematically studying collective effects in a scalable solid-state quantum system, and using them for quantum optical applications in agglomerates of highly-doped nanodiamonds.
Tech Support
Section titled “Tech Support”Original Source
Section titled “Original Source”References
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