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Detection of Glucose Using Diamond Solution-Gate Field-Effect Transistor

MetadataDetails
Publication Date2022-06-29
JournalIEEE Transactions on Electron Devices
AuthorsQianwen Zhang, Xiaohui Chang, Bangqiang Xu, Yanfeng Wang, Dan Zhang
InstitutionsXi’an Jiaotong University, Shaanxi Provincial People’s Hospital
Citations3

The concentration of glucose was detected using an H-terminated diamond solution-gate field-effect transistor (H-diamond SGFET). The linker molecular 1-pyrenebutyric acid-N-hydroxy succinimide ester (Pyr-NHS) was introduced to modify the H-diamond surface. Then, glucose oxidase (GOD) was immobilized on the diamond surface by linker Pyr-NHS. Atomic force microscope and scanning electron microscope measurements confirmed the successful immobilization of Pyr-NHS and GOD enzyme on the H-diamond surface. The concentration of glucose was determined by the shift of gate voltage ( <inline-formula xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”> <tex-math notation=“LaTeX”>${V}{\text {GS}}$ </tex-math></inline-formula> ) in transfer characteristics of H-diamond SGFET. Also, the sensitivity of sensor for glucose detection was obtained as −58.69 mV/ <inline-formula xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”> <tex-math notation=“LaTeX”>${\text {log}}{{10}}$ </tex-math></inline-formula> (glucose concentration) by the slope of fitting curve, which represented the relationship between <inline-formula xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”> <tex-math notation=“LaTeX”>${\Delta {V}}{\text {GS}}$ </tex-math></inline-formula> and logarithmic of glucose with concentration increasing from 1 <inline-formula xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”> <tex-math notation=“LaTeX”>$\times 10^{-{3}}$ </tex-math></inline-formula> to 1 M. The reusability of device was characterized by the transfer properties and small standard deviation (SD) of maximum output current ( <inline-formula xmlns:mml=“http://www.w3.org/1998/Math/MathML” xmlns:xlink=“http://www.w3.org/1999/xlink”> <tex-math notation=“LaTeX”>${I}{\text {DS(max)}}$ </tex-math></inline-formula> ) in four tests, indicating excellent reusability for detection of glucose.

  1. 1998 - Evaluation of a home kit blood glucose monitoring device